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Inicio  /  Coatings  /  Vol: 13 Par: 6 (2023)  /  Artículo
ARTÍCULO
TITULO

Preparation of Nitrogen-Doped ZnFe2O4-Modified Carbon Composite and Its Collaborative Energy Storage Mechanism

Li Wang    
Baobao Li    
Hongyu Bai    
Hong Ding    
Na Xu    
Chaofan Yin    
Jingjing Xiong    
Zhiwei Yang    
Xianfa Rao and Binbin Dong    

Resumen

The pyrolytic carbon of polymer adsorbent resin (SAP) is used as a waste carbon source, which can be used as a porous carbon network via pyrolysis to remove surface sodium carbonate and other substances. In this paper, a ZnFe2O4/nitrogen-doped porous carbon composite was prepared using the template method. Through the high-temperature carbonization of a polymer and crystallization of inorganic elements, the morphology of the composite showed uniform load characteristics. This well-defined structure and morphology facilitate the transport of Li+, enhance the effective contact area with the electrolyte, and provide a wealth of active sites. For the SAP-Fe/Zn anode, at a high current density of 0.1 A g-1, the reversible capacity of the anode reached 753 mAh g-1 after 200 cycles, showing excellent magnification performance. The final modified SAP-Fe/Zn&NC electrode had a reversible capacity of 205.6 mAh g-1 after 1000 cycles at the high current density of 2 A g-1, and the cycle retention rate was as high as 80.7%. The enhanced electrochemical performance can be attributed to the abundant active sites and shortened diffusion pathway of the composite. This ensures adequate conversion reactions during the Li-litization process between Zn, Fe, and Li+, alleviates volume expansion, and prevents comminution/aggregation during long cycles at high current densities.

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